Computer-based learning environments serve as a valuable asset to help strengthen teacher preparation and preservice teacher self-regulated learning. One of the most important advantages is the opportunity to collect ambient data unobtrusively as observable indicators of cognitive, affective, metacognitive, and motivational processes that mediate learning and performance. Ambient data refers to teacher interactions with the user interface that include but are not limited to timestamped clickstream data, keystroke and navigation events, as well as document views. We review the claim that computers designed as metacognitive tools can leverage the data to serve not only teachers in attaining the aims of instruction, but also researchers in gaining insights into teacher professional development. In our presentation of this claim, we review the current state of research and development of a network-based tutoring system called nBrowser, designed to support teacher instructional planning and technology integration. Network-based tutors are self-improving systems that continually adjust instructional decision-making based on the collective behaviors of communities of learners. A large part of the artificial intelligence resides in semantic web mining, natural language processing, and network algorithms. We discuss the implications of our findings to advance research into preservice teacher self-regulated learning.